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Spintronic devices are promising for neuromorphic computing due to their greater energy efficiency, high endurance compared to phase change memory and resistive random-access memory [1]. Popular spintronic memristors involve movement of a domain wall (DW) in a perpendicularly anisotropic (PMA) racetrack to achieve variable conductance to implement synaptic weights for deep neural networks (DNNs). However, energy efficient voltage controlled DW devices driven by spin orbit torque with Neel DW stabilized by Dzyaloshinskii-Moriya interaction show stochastic behavior and therefore provide limited states (see Fig.1 [2]). This is modelled rigorously with micromagnetics.&lt;br/&gt;To work with these DW devices and achieve high testing accuracy, the DNNs need to be trained with specific algorithms. In this study, we propose both in-situ and ex-situ training algorithms of DNN based on 2-, 3- and 5-state DW synaptic devices. For in-situ training, a mixed precision framework [3] is adopted where low precision synaptic conductances are tuned based on the quantized value of high precision gradients. With our quantized training, the learning is able to tolerate large conductance variation without any considerable accuracy loss as the synaptic state changes only few times during the entire training due to large inter-state interval. Thus, high programming noise intrinsic to DW devices is accommodated in the training which reduces the required number of programming pulses and the energy to train a DNN. The programming energy required for a DNN with 5-state DW synapse is found to be 1.25 pJ/image for MNIST digit classification with ~96.7% accuracy shown in Fig.2. Ex-situ training algorithm is also proposed where the DW devices are characterized based on statistics and then the devices characteristic is inputted to the quantized training algorithm as constraints which shows ~95% accuracy for 5-state synapses for large conductance variation. This work will pave the way to implement high accuracy intelligent future battery powered IoT edge devices using DW devices.&lt;br/&gt;&lt;br/&gt;Acknowledgement: NSF grant ECCS: #1954589

![](https://assets.underline.io/uploads/markdown_image/1/image/31364699a8a16e0f648f76850d498230.jpg)

Fig. 1: Stochastic nature of DW devices for voltage control of PMA (Ku) [2]

![](https://assets.underline.io/uploads/markdown_image/1/image/17758a182c49845d7959075dda8cb138.jpg)

Fig. 2: Testing accuracy comparison with proposed training

2022 Joint MMM-INTERMAG

Neuromorphic Learning of a Deep Neural Network with Low Precision and Stochastic Domain Wall Based Memristor

The 15th Joint MMM-INTERMAG Conference (2022 Joint) is sponsored jointly by AIP Publishing and the IEEE Magnetics Society. Members of the international scientific and engineering communities interested in recent developments in fundamental and applied magnetism are invited to attend and contribute to the technical sessions. The technical program will include invited and contributed papers in oral and poster sessions, invited symposia, a plenary session, and an evening session, with about 1500 presentations overall. This Conference provides an outstanding opportunity for worldwide participants to meet their colleagues and collaborators and discuss developments in all areas of magnetism research.

The 2022 Joint Conference will offer both in-person and prerecorded on-demand content.

For tickets to the event, please register at the following link: https://magnetism.org/register

Please register for the Joint MMM-Intermag conference to join the event.

This Conference provides an outstanding opportunity for worldwide participants to meet their colleagues and collaborators and discuss developments in all areas of magnetism research.

Spintronic devices are promising for neuromorphic computing due to their greater energy efficiency, high endurance compared to phase change memory and resistive random-access memory [1]. Popular spintronic memristors involve movement of a domain wall (DW) in a perpendicularly anisotropic (PMA) racetrack to achieve variable conductance to implement synaptic weights for deep neural networks (DNNs). However, energy efficient voltage controlled DW devices driven by spin orbit torque with Neel DW stabilized by Dzyaloshinskii-Moriya interaction show stochastic behavior and therefore provide limited states (see Fig.1 [2]). This is modelled rigorously with micromagnetics. To work with these DW devices and achieve high testing accuracy, the DNNs need to be trained with specific algorithms. In this study, we propose both in-situ and ex-situ training algorithms of DNN based on 2-, 3- and 5-state DW synaptic devices. For in-situ training, a mixed precision framework [3] is adopted where low precision synaptic conductances are tuned based on the quantized value of high precision gradients. With our quantized training, the learning is able to tolerate large conductance variation without any considerable accuracy loss as the synaptic state changes only few times during the entire training due to large inter-state interval. Thus, high programming noise intrinsic to DW devices is accommodated in the training which reduces the required number of programming pulses and the energy to train a DNN. The programming energy required for a DNN with 5-state DW synapse is found to be 1.25 pJ/image for MNIST digit classification with ~96.7% accuracy shown in Fig.2. Ex-situ training algorithm is also proposed where the DW devices are characterized based on statistics and then the devices characteristic is inputted to the quantized training algorithm as constraints which shows ~95% accuracy for 5-state synapses for large conductance variation. This work will pave the way to implement high accuracy intelligent future battery powered IoT edge devices using DW devices. Acknowledgement: NSF grant ECCS: #1954589

![](https://assets.underline.io/uploads/markdown_image/1/image/31364699a8a16e0f648f76850d498230.jpg)

Fig. 1: Stochastic nature of DW devices for voltage control of PMA (Ku) [2]

![](https://assets.underline.io/uploads/markdown_image/1/image/17758a182c49845d7959075dda8cb138.jpg)

Fig. 2: Testing accuracy comparison with proposed training

technical paper

Magnetic skyrmions present interesting and unique pseudo-particle behaviors which arises from their topological protection [1-2]. Key among these behaviors is their resonant dynamics, under microwave fields, which include both breathing and gyration modes. Due to their small size, and magnetic-only contrast of skyrmions, coupled with high frequency dynamics – in the GHz regime – it is challenging to do in-situ measurements on these excitations. This work reports the use of small angle neutron scattering (SANS) to capture the dynamics of hybrid skyrmions stabilized in Fe/Gd multilayers by means of dipolar interactions. Using perpendicular DC fields and in-plane RF fields, we explored the gyration modes of hybrid skyrmions away, below, at, and above resonance [Fig.1(a-d)]. We find the dynamic modes of hybrid skyrmions contribute to the SANS signal in two ways: first, the scattered neutrons incur additional transverse momentum as a result of scattering from a moving source, and second, the gyration skyrmions disrupt ordering of the lattice giving rise to enhancement form-factor scattering. Ferromagnetic resonance measurements confirm the RF and DC field conditions for these gyration modes. Our results offer new insights into the nanoscale dynamics of magnetic skyrmions and present a unique use of SANS to probe magnetization dynamics.

![](https://assets.underline.io/uploads/markdown_image/1/image/a7eefda0d3ae85f8c787ee1cd94ec130.jpg)

Fig.1 2D SANS pattern of magnetic skyrmions under different magnetic fields and excitation frequencies: (a) Static state (H=0, RF=0), (b) below-resonance state (H=150 mT, RF=1.2 GHz), (c) at-resonance state (H=150 mT, RF=1.3 GHz) and (d) above-resonance state (H=150 mT, RF=1.4 GHz). All 2D images are plotted with the same intensity scale.

In-situ GHz Dynamics of Skyrmions Probed with SANS

Skyrmions have clear advantages for future spintronic devices over domain walls in terms of information carrying and storage, however there are still many open questions left and inherent challenges in the transition to applications. Here we study the effect of an additional interfacial spin-transfer torque (ISTT) [1], as well as the well-established spin-orbit torque (SOT), on skyrmion collections [2] – group of skyrmions dense enough that they are not isolated from one another – in magnetic multilayers, by comparing modelling using Boris [3], with experimental results. We show that skyrmion collective motion has additional effects not reproduced when compared to modelled isolated skyrmions [1]. In particular, as the skyrmion collection density increases the effect of local disorder is reduced, leading to reduced threshold current densities, and a sharper dependence of skyrmion Hall Angle (SkHA) on velocity in the depinning regime, in agreement with experimental results. When including both the ISTT and SOT, the small SkHA observed in experiment are in good agreement, also explaining the observed diameter-independent SkHA [4], as seen in Figure 1. Contrary to the model which considers the SOT as the only driving torque, and which predicts a monotonically increasing SkHA with decreasing diameter, inclusion of ISTT results in SkHA closely aligned to experimental results, particularly when the effect of local disorder and skyrmion-skyrmion interactions are taken into account. Our results shed further light on collective current-driven skyrmion motion in magnetic multilayers and highlight the significance of the ISTT in understanding current-driven skyrmion motion in magnetic multilayers.

![](https://assets.underline.io/uploads/markdown_image/1/image/219d9cf02b4f240924efc702e30f317a.jpg)

Figure 1. Collective SkHA dependence on skyrmion diameter for (a) N = 50 Sk/µm2 and (b) N = 100 Sk/µm2. (c) Experimentally obtained SkHA from skyrmion collections with a range of diameters with an average current density of 2×1011 A/m2. The overlaid dashed and solid lines show the ideal isolated skyrmion case – independent of current density – for the SOT and ISTT+SOT, respectively. The solid blue line in panel (b) represents a Savitzky-Golay fit to the simulated skyrmion motion, for a current density of Jc = 2×1011 A/m2.

Collective Skyrmion Motion Under the Influence of an Additional Interfacial Spin-Transfer Torque

Co/Gd based synthetic ferrimagnets have received considerable attention owing to the coexistence of both pronounced spin-orbitronic effects and all-optical switching (AOS), allowing for novel, hybrid devices [1,2]. Previous studies [3,4] have shown that spin-orbit torque (SOT) driven domain wall motion in these 3d-4f ferrimagnets system is most efficient at angular momentum compensation. Following this notion, in this study, we explore the stack engineering of Co/Gd based synthetic ferrimagnets to achieve high SOT driven domain wall motion at room temperature[5]. Here, we experimentally demonstrate that magnetization compensation can be achieved and tuned by varying layer thicknesses in Co/Gd(x)/Co/Gd quadlayer systems (see inset of Fig. 1), which shows AOS in the full range of Gd thickness[5]. Fig. 1 (a) shows the coercivity and polar magneto-optical Kerr effect (MOKE)-signal in such a quadlayer system where the middle Gd layer is wedged. The sign change of the MOKE signal and divergence of the coercivity indicate a compensated system. The CIDWM velocity as a function of Gd thickness of this stack has been investigated, after structuring a series of domain wall conduits from another wedge sample grown in the same batch. In Fig. 1 (b) it can be observed that for low to moderate current densities the optimum in the velocity can be found at compensation. As the current density is increased the optimum in the velocity is found to shift towards larger Gd thicknesses, likely due to the difference in temperature dependence of the magnetization in Co and Gd leading to a shift in the compensation thickness due to joule heating during the applied current pulses. Our study shows a significant improvement of the room temperature domain wall velocity in synthetic ferrimagnetic systems through stack engineering. Further studies to explore the role of the weak exchange link provided by the proximity induced Gd magnetization profile are in progress.

![](https://assets.underline.io/uploads/markdown_image/1/image/abbc4d28d2f8fc22cfb8a86256cef998.jpg)

Fig. 1: Coercivity, polar MOKE signal (a) and current-driven domain wall velocity (b) as a function of Gd thickness in a Pt(4)/Co(0.6)/Gd(x)/Co(0.7)/Gd(1.5) multilayer system (thicknesses in nm in parenthesis), and x indicates Gd layer thickness.

![](https://assets.underline.io/uploads/markdown_image/1/image/439e7460be2e15697bd7be423caa409c.jpg)

Fig. 1 (a) The XRD pattern and (b) the FC magnetic moment as a function of temperature at 100 Oe, of LNMO films. The sample numbers represent the annealing time in minutes.

Fast Current-Induced Domain Wall Motion in Compensated Co/Gd Quadlayers

In recent years, there was an increased interest in using antiferromagnetic (AFM) materials for THz frequency sources. The operation of such AFM structures is based on the AFM resonance, which can have THz frequencies, exceeding the frequency ferromagnetic (FM) resonances by order of magnitude [1,2]. Recent experiments showed that it is possible to generate such signal in AFM FeRh/Pt bi-layers by optically exciting them with a sub-picosecond laser pulse [3]. The signal in the AFM state can be originated from a partial phase transition induced by the laser heat from the AF to the FM phase [4]. Such transformation occurs on a sub picosecond time scale [5-7]. Using atomistic simulations, it is possible to reproduce such transition by including both the bilinear and biquadratic exchanges in the Hamiltonian [7,8]. However, to model larger spatial structures, a coarse-grained model for the dynamic of the magnetization is desirable. Here, we present a micromagnetic formulation to model the magnetization dynamics and phase transition in FeRh at low and high temperatures, including the transition near the Curie temperature. The formulation is based on a mean field approximation (MFA), where each macrospin is modeled by two coupled sublattices, including the atomistic biquadratic interactions described as a micromagnetic inter-sublattice molecular field with a cubic dependence of the magnetization. To validate the model, we compare our simulations of the phase transitions in the static and dynamic case with the existing literature. The results show an agreement with the experiments and atomistic modeling, displaying the characteristic hysteretic behavior for the magnetization (Fig. 1), and a similar dynamic response to an external thermal pulse (Fig.2).

![](https://assets.underline.io/uploads/markdown_image/1/image/514f2aed032312bb7acd410db166547c.jpg)

Equilibrium magnetization as a function of temperature.

![](https://assets.underline.io/uploads/markdown_image/1/image/25e2660f89da1d9cb11ba63fe22f9af2.jpg)

Dynamic response of the magnetization to an optical pulse (shaded area) for different values of the atomistic damping coefficient α

Macromagnetic Simulation of AFM-FM phase transition in FeRh using a modified Landau-Lifshitz-Bloch Equation

Synthetic antiferromagnets (SAFs) are of interest in a wide variety of spintronic applications owing to their net zero magnetisation and inherent tunability arising from control over complex stacking sequences [1]. They show very fast domain wall (DW) motion in response to spin torques [2]. Here we describe current-driven DW motion in an SAF with stack structure Ta/[Ru/Pt/CoB/Ru/Pt/CoFeB]×5/Ru/Pt which displays both perpendicular magnetic anisotropy (PMA) and the Dzyaloshinskii-Moriya interaction (DMI). The alternating CoB and CoFeB layers had their thicknesses adjusted to give net zero magnetisation (as determined by SQUID-VSM) for applied fields up to ~500 Oe. They were patterned into 2 µm wide wires with Cu leads attached to each end. These were fabricated on Si3N4 membranes to permit imaging of DW motion using scanning x-ray transmission microscopy. The distinct chemical composition of the two sublattices means that we could use the element specificity of this technique to observe the CoFeB separately whilst imaging at the Fe L3 edge, whilst contrast at the Co L3 edge is dominated by the other sublattice. Inverted domain structures observed at these two edges, as shown in Fig. 1, confirm the SAF ordering of the layers. Current pulses drive domain wall motion, as shown in Fig. 2, with velocities up to ~ 20 m/s achieved at current densities as low as 4 × 1011 A/m2.

![](https://assets.underline.io/uploads/markdown_image/1/image/d87de30dbef334ff75e4447e90cf2feb.jpg)

Fig. 1: STXM images acquired at zero field the Co and Fe L3 edges, which probe different sublattices of the SAF. A finger-shaped Cu lead is visible on the left. 1 µm scale bar.

![](https://assets.underline.io/uploads/markdown_image/1/image/04b915124bc7866fb80c310fb03a761b.jpg)

Fig. 2: DW velocity against current density measured using 5 ns current pulses.

Current-Driven Domain Wall Motion in a Synthetic Antiferromagnet Multilayer

We show that antiperovskite Mn4N transforms from ferri- to ferromagnetism at room temperature (RT) when the Mn content is decreased by the addition of non-magnetic In atoms. Mn4N films have attracted increasing attention as candidates for the current induced domain wall motion (CIDWM) devices. They have a small magnetization (Ms ~ 100 kA/m [1]) and perpendicular magnetic anisotropy, contributing to high CIDWM mobility with low threshold current. In addition, Mn4-xNixN [2] and Mn4-xCoxN [3] epitaxial films have x-dependent magnetic compensation (MC) points at RT, probed by X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism (XMCD) measurements. In Mn4-xNixN nanowires at the vicinity of the MC, we demonstrated ultrafast and efficient CIDWM (3,000 m/s with j=1.2×1012 A/m2) by pure spin transfer torque at RT [4]. In this work, we focused on Mn4-xInxN epitaxial films as new candidates for such materials [5]. We grew 25nm-thick Mn4-xInxN films (x=0, 0.15 and 0.27) on MgO(001) by MBE. XAS and XMCD measurements were performed at the twin APPLE II undulator beam line BL16A of KEK-PF in Japan. Figure 1 shows XAS and XMCD spectra of Mn-L2,3 absorption edges of the samples. In the XAS spectra of all the samples, distinct shoulders marked by arrows appear at about 2 eV above the main L3 edges, which are caused by fcc-Mn(II) atoms [3]. In the XMCD spectrum of Mn4N(x=0), corner-site Mn(I) and fcc-Mn(II) atoms are attributable to peaks α and β, respectively [3]. Their different signs show that the magnetic moments of Mn(I) and Mn(II) are aligned antiparallel. When the In composition x increases up to 0.27, the sign of peak β reverses while that of peak α remains unchanged. It means that the magnetic moment of Mn(II) reverses and now aligns parallel to that of Mn(I), showing a ferri-to-ferromagnetic transition at RT. Figure 2 shows the anomalous Hall effect (AHE) curves at RT. The sign reversal of ρAHE reconfirms the reversal of the magnetic moment of Mn(II) between x = 0.15 and 0.27 in Fig. 1.

![](https://assets.underline.io/uploads/markdown_image/1/image/26c9e42c0a4ba29f78f74bc6894e54cc.jpg)

Fig. 1 XAS and XMCD spectra at Mn-L2,3edges in (a) Mn4N, (b) Mn3.85In0.15N and (c) Mn3.85In0.27N.

![](https://assets.underline.io/uploads/markdown_image/1/image/cfe5232aa05ae86551424552fbca083a.jpg)

Fig. 2 Anomalous Hall effect curves of Mn4−xInxN (x=0.15 and 0.27) films on MgO(001).

Making ferrimagnetic Mn4N ferromagnetic by non-magnetic element doping

Magnetic domain walls (DWs) in ferromagnetic nanostrips with perpendicular magnetic anisotropy have widely been a subject of research, not only due to its intrinsic fundamental interest but also to develop spintronic devices where information is coded in domains between walls [1,2]. To that purpose, ferrimagnetic materials (FiM) are recently attracting much attention due to their fast DW dynamics, almost zero interaction with external fields and a wide availability in nature. Controlling the current-driven DW along curved FiMs strips is essential to develop DW-based circuitry, but it faces problems such as DW distortion [3]. A proper design for the strip geometry may overcome these problems, as shape is intimately connected with DW motion via spin currents and interfacial phenomena in the structure. Studying the influence of temperature (or composition) is also key for developing real applications. Therefore, understanding the influence of shape and temperature to fully control the DW motion is nowadays a fundamental topic in spintronics research. In this work we perform a micromagnetic (μm) study on DW motion in ring-like FiM strips, characterising DW terminal velocities and inertial times, as a function of temperature, width, curvature of the strip (see insets in Fig. 1(a)) and density currents (J). Our full μm model treats spin dynamics in each sublattice separately, which yields results close to ‘realistic’ FiM. Results show that strips with low width and high curvature give high DW velocities (VDW &gt; 1000 m/s), with ultra-short response times (τ &lt;&lt;0.1 ns, see Fig.1 (b)). This is optimal for developing compact and high-speed tracks for domains since opposite DWs travel at lower but similar speeds, leading to negligible domain distortion. Our results will help to understand curvature effects to develop efficient and reliable DW-based devices.

![](https://assets.underline.io/uploads/markdown_image/1/image/8036e1ee8c0a9ee895bd4c2baa9dc144.jpg)

Fig.1. (a) DW velocity as a function of J from sub-lattice i = 1 in a FiM strip of width w = 256 nm and different effective radius re (nm) at the angular momentum compensation temperature TA = 260 K. (b) Instantaneous DW velocities for three values of J and for a curved strip of re = 384 nm and w = 256 nm at T = TA. Relaxation times (τ) are extracted from the equation (solid curve) fitted to the data (symbols).

Current-Driven Domain Wall Motion in Curved Ferrimagnetic Strips Above and Below the Angular Momentum Compensation

Recent years have seen an increase of interest in the dynamics of ferrimagnetic materials, in particular in the motion of domain walls [1-4]. Ferrimagnetic materials represent unique systems where the ease of manipulating the spins with applied magnetic fields is combined with exchange-driven acceleration of the internal spin dynamics. Of particular interest is the temperature range around the magnetic and spin compensation points, finely balancing both magnetic moment and angular momentum of the system, and leading to a very particular character of magnetic switching by the domain wall motion. Here we present our studies of the temperature-dependent domain wall dynamics in the temperature range covering both angular momentum and magnetization compensation points in garnet film, and reaching up to the Curie temperature [5]. This is made possible by the very low coercive field of the material, not exceeding 5 mT even in the close vicinity of magnetization compensation temperature. The sample used in our experiments is a single-crystal thin film of magnetic garnet. A very unusual behavior of the domain-wall dynamics is observed, such as extraordinarily high mobility of the domain walls at very low fields. Drastic changes of both domain-wall velocity and mobility by more than 2 orders of magnitude are observed across a relatively small temperature range, related to the delicate balance of magnetization and spins of iron and rare-earth sublattices [5]. Therefore, such fine tuning of the corresponding momenta could be the key for developing ultrafast ferrimagnetic spintronic devices. The work was supported by the Russian Foundation for Basic Research (Projects No. 18-52-16006, 18-29-27020) and the Government of the Russian Federation (Project No. 075-15-2019-1874).

Domain wall dynamics across magnetic and spin compensation points in ferrimagnets

Topological spin structures, such as domain walls (DW) and skyrmions, have intriguing features and can play a key role in spintronics. In both ferromagnets (FM) and antiferromagnets (AFM) a DW, driven by applied torque, behaves like a solid particle, which can be described by collective variables: DW position and the angle of the magnetic order vector, albeit the dynamic properties are dramatically different. For an AFM the DW energy as a function of its momentum is the same as that of a standard relativistic particle (Fig. 1), because of the Lorentz invariance of the AFM dynamics [1]. For FMs the gyrotropic dynamic term couples two degrees of freedom that slows down a FM DW and results in the periodic dependence of the DW energy on momentum (Fig. 1). Thus, the AFM DW is stable up to higher speeds (~10km/s in contrast to ~100m/s for FMs). We demonstrate that the DW dynamics in ferrimagnetic (FiM) materials near the spin compensation point is entirely different from the FM and AFM cases [2]. The dispersion law for FiM DWs exhibits two crossed branches with opposite group velocities (Fig. 1), where each branch contains an endpoint [3]. Driven by a field-like torque, a FiM DW accelerates to a higher speed and momentum than its FM counterpart [4] and can reach the endpoint. Wherein it falls into a region of instability, where the internal dynamics of the DW is excited, and the collective variables approach fails. We show by micromagnetic simulations that the dynamical state of a DW in this case covers a wide frequency range, far beyond the magnon bandgap of a FiM. In this way the FiM DW driven by external field-like torque acts as an efficient source of the spin waves (SW), propagating out of the DW region. We show that by varying the applied torque and spin uncompensation of a FiM one can reach three qualitatively different regimes of the excited SWs: i) frequency-comb spectrum, shown in Fig.2, ii) chaotic behavior of the DW with the broad SW spectrum, iii) double-frequency SW excitation.

![](https://assets.underline.io/uploads/markdown_image/1/image/d58bb938c75083b271d7c47eff1fa103.jpg)


Fig.1 Dependence of the energy on momentum for a DW in FM, AFM (gray), and FiM near compensation point (blue) nano-strips.

![](https://assets.underline.io/uploads/markdown_image/1/image/60b60e08628ebcc51a436f9ca0f5c150.jpg)

Fig.2 Spectra of the dynamic state inside the DW (a) and magnons emitted outside (b).

Nonstationary domain wall dynamics in almost compensated ferrimagnets: a novel scenario

In recent years, current-induced domain wall motion (CIDWM) is attractive research field in spintronics because it’s expected to enable magnetic non-volatile memory. Our group focuses on Mn4N and its based nitrides as new candidates for CIDWM application. Especially, Mn4-xNixN nanowire recorded a DW velocity of 3,000 m/s only by spin-transfer torque [1]. We attributed this to the compensation of Mn4-xNixN around x=0.2 [2]. In spite of the excellent CIDWM, magneto-transport properties in Mn4-xNixN have scarcely been reported. In this work, we report both experimental and theoretical investigations of these properties with anisotropic magnetoresistance (AMR) measurement and calculation of PDOS with Vienna Ab initio Simulation Package (VASP). Figure 1 shows Fourier coefficients of AMR measurements in Mn4-xNixN on SrTiO3(001) substrates and energy state of d electrons under various crystal fields. C2 represents the coefficient of cos2θ component and C4 does that of cos4θ, where θ is the angle made by the current and the magnetization. Above 100K, small C2 components dominate AMR while C4 drastically became large below 100K. This represents the emergence of the tetragonal-like crystal field below 100K because it depends on the difference in PDOS between dxy and dyz, dzx states [3]. However, this trend was weakened by large Ni composition. Figure 2 shows PDOSs of d orbitals in Mn and Ni at corner site (I-site) in Mn4-xNixN (x=0, 0.5). By Ni substitution, spin polarization of d orbitals decreased at Fermi level (EF). This leads to decrease in both AMR ratio and C4 components, derived from the theory of s-d scattering [4]. In the previous study, the emergence of C4 components in Mn4N was attributable to the possible external effect such as lattice strain caused by the thermal expansion [3,4]. However, since all structures were set to be cubic in our calculation, we expect this is attributable to intrinsic change in PDOS, and dramatically affected by Ni doping. In the talk, we’re going to further investigate the modulation of Hall effect in Mn4-xNixN by Ni composiiton.

![](https://assets.underline.io/uploads/markdown_image/1/image/733d7a68846d668c0d9e1632ad6ca552.jpg)

Fig. 1 Fourier coeffcients of AMR in Mn4-xNixN and energy state of d orbitals.


![](https://assets.underline.io/uploads/markdown_image/1/image/df111606651ce41db44558dbc23cd7fa.jpg)


Fig. 2 PDOS of d orbitals of Mn at corner site in Mn4-xNixN (x=0, 0.5)

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